[DFTB-Plus-User] Convergence issues in DFTB+ calculations?

Hemanth Haridas hemanth.h at iitgn.ac.in
Thu Jun 1 08:15:29 CEST 2023


I am trying to calculate the Fermi level of a DNA-graphene system. I was
able to get the calculations for graphene and DNA strand to converge
separately. However, when I try to calculate the same for the DNA-graphene
system, the SCC cycles do not converge even after multiple restarts. Any
information on why this is happening would be much appreciated.

Input file is attached

Geometry = {
	TypeNames = { "C" "P" "N" "O" "H"}
	TypesAndCoordinates [Angstrom] = {
         1      -14.24500       15.63300       -0.87000
         1      -14.26200       14.28700        2.62100
         1      -14.25400       11.44000       -1.29500
         1      -14.23200       10.08800        2.10000
         1      -14.23000       12.80400       -1.22100
         1      -14.26000       12.86700        2.45800
         1      -13.00900       13.51800       -1.11900
         1      -13.08200       12.21200        2.35700
         1      -13.01000       14.94300       -0.90000
         1      -13.04100       15.00200        2.75300
         1      -11.78600       15.67500       -0.83800
         1      -11.80700       14.30700        2.72800
         1      -14.25400        7.26900       -1.96000
         1      -14.19300        5.88300        1.67700
         1      -14.22300        8.70100       -1.83000
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         1      -12.98700        9.37800       -1.67400
         1      -12.99300        7.98800        1.81700
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         1      -13.06200       10.81500        2.22400
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         1      -14.25200       -8.32000       -2.17700
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         1      -13.03500       -7.64000       -2.19300
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         1       -4.45500       -8.64500        6.07900
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         1        7.75900       12.51800        6.30200
         1        8.99300       13.26200        6.30100
         1        8.99400       14.58200        6.29500
         1       10.17000       15.31700        6.15100
         1       -6.93200      -17.11700        6.21400
         1       -5.71500      -16.38200        6.28900
         1       -5.67700      -14.93500        6.15300
         1       -4.48000      -14.24500        6.30700
         1       -4.49700      -12.88200        6.21600
         1       -3.25300      -12.20100        6.35000
         1       -3.19200      -10.78500        6.42300
         1       -2.02600      -10.02600        6.47600
         1       -2.02400       -8.57400        6.47400
         1        6.51300        4.75000        5.75400
         1        6.57200        6.10800        5.94100
         1        7.79400        6.83600        5.97800
         1        7.76200        8.28300        6.03400
         1        8.96200        8.98600        5.92200
         1        8.98400       10.40000        6.02200
         1       10.21600       11.11700        5.93000
         1       10.21500       12.53200        6.11300
         1       11.43500       13.19900        6.06500
         1       11.39800       14.60600        5.98200
         1       12.66500       15.34200        5.85900
         1       -4.49700      -17.06100        6.48100
         1       -3.23800      -16.36800        6.51300
         1       -3.24000      -14.97500        6.52500
         1       -2.01400      -14.30900        6.53500
         1       -2.04300      -12.86300        6.47000
         1       -0.82700      -12.16700        6.49900
         1       -0.80900      -10.74300        6.57900
         1        0.37100      -10.02800        6.49300
         1        7.77600        2.58700        5.76800
         1        7.72600        3.97900        5.74900
         1        8.95400        4.73300        5.71500
         1        8.98100        6.15100        5.84100
         1       10.21900        6.86300        5.73500
         1       10.19800        8.28600        5.76900
         1       11.42200        8.98800        5.73300
         1       11.39000       10.39200        5.80800
         1       12.66400       11.03200        5.77800
         1       12.64600       12.47300        5.89800
         1       13.87200       13.18200        5.77900
         1       13.91100       14.61600        5.80300
         1       -1.98600      -17.05600        6.65900
         1       -0.78000      -16.33300        6.73600
         1       -0.75900      -14.94900        6.72800
         1        0.43800      -14.23300        6.75400
         1        0.40700      -12.81400        6.68300
         1        1.65100      -12.08600        6.67900
         1        1.62500      -10.65400        6.55300
         1        2.85400       -9.95600        6.71000
         1        2.83000       -8.52700        6.61900
         1        4.08800       -7.80900        6.63100
         1        8.93300        0.46100        5.82100
         1        8.95500        1.90900        5.77600
         1       10.19200        2.59900        5.71500
         1       10.17400        4.01200        5.64700
         1       11.44000        4.71600        5.55000
         1       11.45000        6.09400        5.64800
         1       12.62100        6.82500        5.53400
         1       12.60500        8.25100        5.60500
         1       13.84200        8.92100        5.61500
         1       13.86700       10.33200        5.74700
         1        0.39600      -17.05900        6.74600
         1        1.63500      -16.38500        6.81800
         1        1.67300      -14.92100        6.83700
         1        2.82300      -14.18800        6.91300
         1        2.83100      -12.81800        6.89400
         1        3.99400      -12.13500        6.94000
         1        4.04900      -10.71400        6.82400
         1        5.27600      -10.06400        6.77200
         1        5.26700       -8.64600        6.80300
         1        6.46400       -7.93600        6.73900
         1        6.52800       -6.56400        6.68000
         1        7.72700       -5.82400        6.56700
         1        7.72600       -4.43200        6.55700
         1        8.90000       -3.70200        6.29200
         1        8.90400       -2.31600        6.14500
         1       10.11000       -1.59600        5.85000
         1       10.11900       -0.19400        5.87200
         1       11.39600        0.53400        5.71000
         1       11.39500        1.90800        5.56800
         1       12.66200        2.62600        5.50000
         1       12.65100        4.04200        5.42200
         1       13.88000        4.68700        5.35000
         1       13.87200        6.10000        5.43400
         1        2.85700      -17.08500        6.91200
         1        4.04800      -16.33800        7.03200
         1        4.03600      -14.90300        7.03100
         1        5.25900      -14.22200        7.10200
         1        5.22900      -12.83200        7.03300
         1        6.47500      -12.17000        6.97100
         1        6.50300      -10.77200        6.87000
         1        7.68500      -10.05000        6.88400
         1        7.66700       -8.65500        6.83400
         1        8.93700       -7.96100        6.73800
         1        8.94100       -6.52700        6.61500
         1       10.18600       -5.84600        6.46600
         1       10.20500       -4.42900        6.30900
         1       11.33100       -3.73800        5.99700
         1       11.30500       -2.32100        5.74200
         1       12.56000       -1.61000        5.73100
         1       12.59700       -0.19000        5.65000
         1       13.82500        0.49100        5.60100
         1       13.80700        1.89700        5.43400
         1        5.27400      -17.05900        6.97700
         1        6.51700      -16.39500        7.07200
         1        6.49700      -14.93100        7.13400
         1        7.72400      -14.24400        7.19600
         1        7.71100      -12.89000        7.05900
         1        8.92900      -12.14900        7.04700
         1        8.91200      -10.75900        6.96400
         1       10.16800      -10.10900        6.94000
         1       10.17000       -8.67700        6.83700
         1       11.37100       -7.98100        6.63100
         1       11.43100       -6.59800        6.42800
         1       12.59700       -5.86700        6.14600
         1       12.58300       -4.45500        5.93100
         1       13.79400       -3.70800        5.88400
         1       13.81300       -2.31200        5.68200
         1        7.68400      -17.05100        7.19000
         1        8.92600      -16.34500        7.21300
         1        8.95400      -14.94400        7.22400
         1       10.18600      -14.25000        7.26500
         1       10.15600      -12.86100        7.19500
         1       11.38900      -12.20300        7.05700
         1       11.42600      -10.78300        6.94500
         1       12.64600      -10.02600        6.85300
         1       12.61000       -8.66700        6.65500
         1       13.86300       -7.96300        6.36900
         1       13.82800       -6.52600        6.18600
         1       10.14400      -17.08100        7.19300
         1       11.39000      -16.39000        7.23300
         1       11.40000      -14.96100        7.21200
         1       12.66000      -14.29000        7.07100
         1       12.63500      -12.89800        6.99200
         1       13.87300      -12.19400        6.84400
         1       13.82100      -10.76300        6.71900
         1       12.61700      -17.09400        7.21800
         1       13.83000      -16.42000        7.23500
         1       13.85100      -14.99600        7.07000
         5       -4.71800        4.13600       -5.58900
         4       -4.76700        5.00700       -5.18900
         1       -5.07900        4.78700       -3.78500
         5       -6.10700        5.11700       -3.67000
         5       -4.41500        5.42900       -3.09600
         1       -5.21300        3.24900       -3.46700
         5       -5.54100        3.15600       -2.44700
         4       -6.31000        2.62400       -4.23400
         1       -5.87400        1.43100       -4.85300
         5       -6.11400        0.59200       -4.22600
         3       -6.57700        1.37300       -6.17400
         1       -6.44200        2.44000       -7.00200
         5       -5.75300        3.23000       -6.62700
         1       -7.54500        0.41300       -6.36000
         4       -7.96900       -0.34500       -5.48800
         3       -8.05300        0.47200       -7.65000
         5       -8.49600       -0.37400       -8.05800
         1       -7.69000        1.34700       -8.66600
         4       -8.00500        1.14100       -9.83100
         1       -6.97300        2.48700       -8.22800
         1       -6.77200        3.77600       -9.03600
         5       -7.60400        4.47700       -8.79100
         5       -6.66100        3.57000      -10.11300
         5       -5.83700        4.33100       -8.78600
         1       -4.40900        1.59300       -4.99800
         5       -4.14000        2.19100       -5.86200
         5       -3.91500        0.65400       -5.05200
         1       -3.98400        2.27200       -3.71300
         5       -3.01000        2.81300       -3.93700
         4       -3.85000        1.28700       -2.63000
         2       -2.68400        1.58200       -1.58000
         4       -1.40600        1.54500       -2.31600
         4       -3.03400        2.76100       -0.80600
         4       -2.76300        0.30200       -0.71000
         1       -3.85200        0.09400        0.12500
         5       -4.84200        0.26100       -0.43900
         5       -3.84800        0.76800        1.01000
         1       -3.98700       -1.33900        0.67800
         5       -4.98000       -1.59800        0.90900
         4       -3.50300       -2.38400       -0.21300
         1       -3.38300       -3.58400        0.57800
         5       -4.29500       -4.13300        0.21200
         3       -2.05300       -4.29400        0.12300
         1       -1.01200       -4.35400        0.93500
         5       -0.99200       -3.76900        1.83500
         1       -1.94400       -4.73800       -1.14300
         4       -2.80100       -4.53600       -2.02100
         3       -0.83800       -5.49700       -1.38500
         5       -0.62400       -5.69200       -2.34900
         1        0.30300       -5.43900       -0.61900
         4        1.41700       -5.67600       -1.13700
         1        0.09900       -5.03400        0.68800
         1        1.16900       -5.23200        1.75500
         5        1.96300       -5.93900        1.46800
         5        0.72500       -5.49200        2.77500
         5        1.62800       -4.21600        1.93900
         1       -3.50500       -3.09500        2.03000
         5       -2.81600       -3.53500        2.78500
         5       -4.57100       -3.34200        2.31700
         1       -3.20800       -1.66400        1.89200
         5       -2.16300       -1.37100        1.60100
         4       -3.79400       -0.98400        3.02100
         2       -2.94300       -0.03000        3.92200
         4       -1.58300       -0.65400        4.26800
         4       -3.01000        1.29300        3.28700
         4       -3.77100        0.06400        5.24000
         1       -4.47400       -1.04600        5.71800
         5       -4.09400       -2.08800        5.46600
         5       -5.45600       -0.98000        5.21100
         1       -4.53200       -0.96800        7.23100
         5       -3.51100       -0.76000        7.64400
         4       -5.43100        0.09600        7.50900
         1       -6.04300       -0.19800        8.79400
         5       -5.60500        0.60100        9.43700
         3       -7.46000       -0.24100        8.63500
         1       -8.15400       -1.37900        8.69700
         5       -7.64000       -2.30900        8.68300
         1       -8.03700        1.00200        8.52100
         4       -7.43700        2.05400        8.69500
         3       -9.45400        0.91100        8.28300
         5       -9.94900        1.79600        8.19200
         1      -10.19300       -0.14800        8.32100
         4      -11.39000       -0.02200        8.17600
         1       -9.48300       -1.46900        8.61100
         1      -10.30300       -2.63600        8.95700
         5      -11.23200       -2.59200        8.33100
         5      -10.59400       -2.68200        9.97600
         5       -9.75900       -3.53900        8.74100
         1       -5.38800       -1.49600        9.27000
         5       -5.92700       -2.02100       10.10500
         5       -4.42700       -1.19600        9.70900
         1       -5.17800       -2.25700        7.93400
         5       -6.05000       -2.54600        7.28900
         4       -4.13800       -3.27300        8.05000
         5       -3.32200       -2.92800        7.68000
	}
	Periodic = Yes
	LatticeVectors [Angstrom] = {
		29.50000000        0.00000000        0.00000000
      		0.00000000       34.50000000        0.00000000
      		0.00000000        0.00000000       15.00000000 	
	}
}

Driver = {}

Hamiltonian = DFTB {
        Scc = Yes
        ThirdOrder = Yes
        MaxSCCIterations = 200
        ReadInitialCharges = Yes
        HubbardDerivs = {
                O = -0.19
                H = -0.16
                P = -0.14
                N = -0.13
                C = -0.23
        }
        SlaterKosterFiles = Type2FileNames {
                Prefix  = "./mio-1-1/"
                Separator = "-"
                Suffix = ".skf"
                LowerCaseTypeName = No
        }
        Filling = Fermi {
                Temperature [K] = 300.0
        }
        MaxAngularMomentum = {
                P = "d"
                O = "p"
                C = "p"
                H = "s"
                N = "p"
        }
        KPointsAndWeights = SupercellFolding {
                10 0 0
                0 10 0
                0 0 1
                0.5 0.5 0.0
        }
}


-- 
*Hemanth H 18310019*
Research Scholar
IIT Gandhinagar
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